Title | Nitrogen-Doped Graphene as Efficient Metal-Free Electrocatalyst for Oxygen Reduction in Fuel Cells |
Creator | |
Date Issued | 2010-03 |
Source Publication | ACS NANO Impact Factor & Quartile |
language | 英语 |
Original Document Type | Article |
Keyword | graphene N-doping oxygen reduction fuel cell |
WOS Keyword | CHEMICAL-VAPOR-DEPOSITION ; WALL CARBON NANOTUBES ; FILMS ; SHEETS ; NANOCOMPOSITE ; ELECTRODES ; GRAPHITE ; CRYSTALS ; SINGLE |
Abstract | Nitrogen-doped graphene (N-graphene) was synthesized by chemical vapor deposition of methane in the presence of ammonia. The resultant N-graphene was demonstrated to act as a metal-free electrode with a much better electrocatalytic activity, long-term operation stability, and tolerance to crossover effect than platinum for oxygen reduction via a four-electron pathway in alkaline fuel cells. To the best of our knowledge, this is the first report on the use of graphene and its derivatives as metal-free catalysts for oxygen reduction. The important role of N-doping to oxygen reduction reaction (ORR) can be applied to various carbon materials for the development of other metal-free efficient ORR catalysts for fuel cell applications, even new catalytic materials for applications beyond fuel cells. |
Funding Project | National Research Foundation of Korea [R31-2008-000-20012-0] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS) |
Publisher | AMER CHEMICAL SOC |
Publication Place | WASHINGTON |
ISSN | 1936-0851 |
EISSN | 1936-086X |
Volume | 4Issue:3Pages:1321-1326 |
DOI | 10.1021/nn901850u |
Page Number | 42 |
WOS Subject | Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary |
WOS Research Area | Chemistry ; Science & Technology - Other Topics ; Materials Science |
WOS ID | WOS:000275858200010 |
Indexed By | SCIE ; EI ; SCOPUS |
EI Accession Number | 20101312816051 |
EI Keywords | Graphene |
URL | 查看原文 |
PubmedId | 20155972 |
scopuseid | 2-s2.0-77950140364 |
ESI Hicited Paper | 2020-01 ; 2020-03 ; 2020-05 ; 2020-09 ; 2020-11 ; 2021-01 ; 2021-03 |
User Journal Classification | T3(B)类 |
Corresponding author address | [Liu, Yong]Biomedical Engineerig Academy,School of Ophthalmology and Optometry,Wenzhou Medical College,270 Xueyuan Road,China |
scopus subject classification | Materials Science (all);Engineering (all);Physics and Astronomy (all) |
Top Journal | TOP期刊 |
Citation statistics | |
Document Type | Journal article |
Identifier | https://kms.wmu.edu.cn/handle/3ETUA0LF/10257 |
Collection | Wenzhou Medical University |
Corresponding Author | Liu, Yong |
Affiliation | 1.Department of Chemistry,School of Science,Beijing Institute of Technology,China; 2.Biomedical Engineerig Academy,School of Ophthalmology and Optometry,Wenzhou Medical College,270 Xueyuan Road,China; 3.School of Energy Engineering,Ulsan National Institute of Science and Technology (UNIST),No. 685 Namyoedong,South Korea; 4.Department of Chemical Engineering,Case Western Reserve University,10900 Euclid Avenue,United States |
Recommended Citation GB/T 7714 | Qu, Liangti,Liu, Yong,Baek, Jong-Beom,et al. Nitrogen-Doped Graphene as Efficient Metal-Free Electrocatalyst for Oxygen Reduction in Fuel Cells[J]. ACS NANO,2010,4(3):1321-1326. |
APA | Qu, Liangti, Liu, Yong, Baek, Jong-Beom, & Dai, Liming. (2010). Nitrogen-Doped Graphene as Efficient Metal-Free Electrocatalyst for Oxygen Reduction in Fuel Cells. ACS NANO, 4(3), 1321-1326. |
MLA | Qu, Liangti,et al."Nitrogen-Doped Graphene as Efficient Metal-Free Electrocatalyst for Oxygen Reduction in Fuel Cells".ACS NANO 4.3(2010):1321-1326. |
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